Suggestions by @jesselee

Paul Bunyan

as Paul Bunyan in The Mr Men Movie

Shere Khan

as Shere Khan in The Mr Men Movie

Magneto (Erik Lehnsherr)

as Magneto in The Mr Men Movie

Sabretooth (Victor Creed)

as Sabrertooth in The Mr Men Movie

Sabertooth

as Sabretooth in The Mr Men Movie

Madame Medusa

as Madame Medusa in The Mr Men Movie

Madame Hydra/Viper

as Madame Viper / Hydra in The Mr Men Movie

Judge Claude Frollo

as Claude Frollo in The Mr Men Movie

White Queen (Emma Frost)

as Emma Frost in The Mr Men Movie

Galactus

as Galactus in The Mr Men Movie

Doctor Victor von Doom

as Doctor Doom in The Mr Men Movie

Venom

as Venom in The Mr Men Movie

Carnage (Cletus Kasady)

as Carnage in The Mr Men Movie

Green Goblin (Norman Osborn)

as Green Goblin (Norman Osborn) in The Mr Men Movie

Prince Phillip

as Prince Phillip in The Mr Men Movie

Tiger Lily

as Tiger Lily in The Mr Men Movie

Queen of Hearts

as Queen of Hearts in The Mr Men Movie

Finn Mertens (Finn the Human)

as Finn the Human in The Mr Men Movie

Tinker Bell (Disney Character)

as Tinker Bell in The Mr Men Movie

Mushu

as Mushu in The Mr Men Movie